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Oddly enough, i have trouble connecting to that over IPv6 too. Even though me and my nearest Akamai PoP are probably far away from the Let’s Encrypt validation systems.
(IPv4 works.)
You might need to contact Akamai?
I also get a “503”, “Service Unavailable - DNS” from http://dcv.akamai.com/ (which is IPv4-only anyway) but that might be normal. (They probably deleted that validation file immediately after it failed.)
Edit: Akamai’s using anycast for those 2 IPs, and it looks like they’re returning the same 2 IPs regardless of location. Maybe it’s a routing issue specific to that address (range) rather than some sort of issue specific to one region.